A highly tunable phosphine–imine ligand family is introduced. Following metallation with ruthenium, deprotonation of the ligand affords a phosphine–enamido species. Complexes with the ligand in both the imine and enamido forms are active toward acceptorless dehydrogenation reactions.
J. M. Stubbs, K. F. Firth, B. J. Bridge, K. J. Berger, R. J. Hazlehurst, P. D. Boyle and J. M. Blacquiere, Dalton Trans., 2017, 46, 647 DOI: 10.1039/C6DT04088H
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