Selective catalytic reduction of NO by cerium-based metal–organic frameworks

Simon Smolders; Jannick Jacobsen; Norbert Stock; Dirk De Vos

doi:10.1039/C9CY02029B

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Selective catalytic reduction of NO by cerium-based metal–organic frameworks†

Simon Smolders,

^a Jannick Jacobsen,^b Norbert Stock

^b and Dirk De Vos

*^c

Author affiliations

* Corresponding authors

^a Centre for Membrane Separations, Adsorption, Catalysis and Spectroscopy for Sustainable Solutions, KU Leuven, Celestijnenlaan 200F P.O. Box 2454, 3001 Leuven, Belgium

^b Institut für Anorganische Chemie, Christian-Albrechts-Universität, Max-Eyth Straβe 2, 24118 Kiel, Germany

^c Centre for Surface Chemistry and Catalysis, Belgium
E-mail: dirk.devos@kuleuven.be

Abstract

Cerium oxide clusters have been incorporated in a porous metal–organic framework to increase their activity for the selective catalytic reduction (SCR) of NO with NH₃. In addition, a new set of bimetallic MOFs, Ce_x/Zr-CAU-24, was synthesized to further enhance the acid properties and thus increase the SCR activity of the cerium sites.

This article is part of the themed collection: Catalysis Science & Technology 10th Anniversary Symposium

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Article information

DOI: https://doi.org/10.1039/C9CY02029B
Article type: Communication
Submitted: 09 oct. 2019
Accepted: 13 dic. 2019
First published: 17 dic. 2019

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Catal. Sci. Technol., 2020,10, 337-341

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Selective catalytic reduction of NO by cerium-based metal–organic frameworks

S. Smolders, J. Jacobsen, N. Stock and D. De Vos, Catal. Sci. Technol., 2020, 10, 337 DOI: 10.1039/C9CY02029B

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Catalysis Science & Technology

Selective catalytic reduction of NO by cerium-based metal–organic frameworks†

Abstract

Supplementary files

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Selective catalytic reduction of NO by cerium-based metal–organic frameworks

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