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Herein, a series of twisted graphene-like MOFs (TGL-MOFs) with controlled interlayer twisted angle were constructed. Benefiting from the optimized electronic structure and improved charge separation ability, the TGL-MOF demonstrated switchable CO/CH4 product selectivity via CO2 photoreduction.
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H. Zhang, Z. Peng, W. Yuan, B. Li and Q. Zhai, Chem. Commun., 2026, Accepted Manuscript , DOI: 10.1039/D6CC02843H
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