We present a covalent amidation strategy for assembing biohybrids from CdS@SiO₂ core-shell spheres and microorganisms. Encapsulation CdS within SiO₂ layer significantly reduces cellular damage, while amidation creates robust bio-abiotic interfaces for efficient electron/mass transfer. This enhances biocompatibility and improves the H₂ or CH₄ production of the biohybrid systems.
J. Mi, W. Chen, J. Li, L. Liu, Z. Yuan, J. Liu and Y. Yong, Chem. Commun., 2026, Accepted Manuscript , DOI: 10.1039/D6CC00563B
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