USY zeolites with tailored silica-to-alumina ratios (SAR = 5–120) were prepared via steam-acid leaching. Increasing SAR concurrently generates hierarchical mesoporosity and shifts the framework from hydrophilic to hydrophobic. This work establishes a dual-control adsorption mechanism, providing a rational design blueprint for FAU-type zeolites in VOC molecular separation and capture.
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J. Wang, L. Li, L. Li, C. Liu, R. Bai and P. Liu, Chem. Commun., 2026, Accepted Manuscript , DOI: 10.1039/D6CC00275G
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