We report a 2D coordination solid, (pyz)FeCl2, that combines semiconducting and magnetic properties. It exhibits a ∼1.0 eV band gap, high-spin Fe2+, and strong, stable photoconductivity with thermally activated, spin-dependent transport. Its robust stability and coupled spin–charge–light responses highlight its promise for next-generation 2D magneto-optoelectronic devices.
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M. S. Lassoued, X. Huang, A. Hussain and Y. Zheng, Chem. Commun., 2026, Advance Article , DOI: 10.1039/D5CC06087G
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