Design of nonlinear metastructure for temperature detection and biosensing based on second harmonic generation in theory

Abstract

When the second harmonic generation (SHG) occurs in temperature-controlled ferroelectric crystals, it serves as an effective method for detecting temperature and changes in refractive index (RI). A one-dimensional nonlinear metastructure (NM) composed of periodically poled lithium niobate crystals is designed precisely to exhibit significant SHG enhancement in the visible to near-infrared spectral range. When a tunable fundamental electromagnetic wave is incident at a frequency (f) near 241 THz, the NM achieves frequency conversion and enables wide-range temperature detection (25 °C~105 °C) at the second harmonic wave (SHW) scale 2f with a sensitivity of S=0.32 %/°C. By altering the filling material of the sample layer, it is possible to distinguish between three types of healthy or cancerous liver tissues using RI biosensing with a fundamental wave around 273 THz. The sensing range is from 1.3463~1.3655, with a S of 14.75 THz/RIU. The proposed NM integrates the SHW effect with optical detection and sensing, offering new insights for SHW applications and biomedical fields.

Supplementary files

Article information

Article type
Paper
Submitted
07 Apr 2025
Accepted
12 May 2025
First published
13 May 2025

J. Mater. Chem. B, 2025, Accepted Manuscript

Design of nonlinear metastructure for temperature detection and biosensing based on second harmonic generation in theory

C. Yang, Y. Wei, H. Liu, X. Li and H. Zhang, J. Mater. Chem. B, 2025, Accepted Manuscript , DOI: 10.1039/D5TB00794A

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