Here, we present the first Co(III) catalysed efficient metal ligand cooperative route for the synthesis of quinazolinone using acceptorless dehydrogenation of primary alcohols. An air-stable phosphine-free Co(III) complex anchored by a hexadentate ligand was efficiently utilized in the synthesis of a wide variety of quinazolinone derivatives (28 examples).
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P. Kukreti, T. Patnaik, R. Chauhan, K. Sharma, R. Saini and K. Ghosh, Org. Biomol. Chem., 2025, Accepted Manuscript , DOI: 10.1039/D5OB01916H
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