Thermal transport properties of graphene aerogel as an advanced carrier for enhanced energy storage

Abstract

Leveraging graphene aerogels as carriers offers innovative avenues for achieving enhanced energy density, thermal conductivity, and stability in energy storage materials due to their unique attributes. This study investigates the thermal transport properties of composite sulfur cathode materials and phase change materials based on graphene aerogels using molecular dynamics simulation. A graphene aerogel model is established, and the effects of sulfur and octadecane content on the thermal transport properties of graphene aerogels and graphene aerogel-based composites are examined. A theoretical model of heat transport is developed to analyze the contribution of fillers and graphene aerogels to the thermal conductivity of the composites. The results show that the theoretical analytical model shows strong agreement with the molecular dynamics results, especially at high filler content. This research provides valuable theoretical guidance for understanding the thermal transport properties of graphene aerogel-based composite sulfur cathode materials and phase change materials.