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Abstract | Cited by

Mixtures containing ammonia-borane and sec-butylamine-borane remain liquid throughout the hydrogen release process that affords tri(N-sec-butyl)borazine and polyborazylene. Concentrated solutions with metal catalysts afford >5 wt% H2 in 1 h at 80 °C and addition of (EMIM)EtSO4 ionic liquid co-solvent eliminates competing formation of insoluble linear poly(aminoborane) (EMIM = 1-ethyl-3-methyl-imidazolium).

Graphical abstract: Transition metal catalysed dehydrogenation of amine-borane fuel blends

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