Modern valence bond theory, in its spin-coupled form, is used to describe the bonding in o- and m-phenylenedimethylidenes and, in particular, to rationalize the different relative stabilities of the quintet states and lower spin multiplicities.
B. Friis-Jensen, D. L. Cooper, S. Rettrup and P. B. Karadakov, J. Chem. Soc., Faraday Trans., 1998, 94, 3301 DOI: 10.1039/A804983A
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