Persistent Photoconductivity Enables In-Sensor Binarization and Reservoir Computing in a Single Organic Phototransistor

Abstract

The persistent photoconductivity (PPC) effect in organic phototransistors (OPTs) offers a promising platform for in-sensor reservoir computing (RC). However, the non-uniform wavelength-dependent spectral response of OPTs, while a valuable resource for RC dynamics, poses a challenge for traditional binarization encoding. In this work, we reframe this non-uniformity as a computational resource. We demonstrate that the device’s non-uniform PPC decay dynamics can be directly harnessed to resolve this contradiction. This physical process, which we term time-dependent binarization (TDB), intrinsically performs channel-adaptive thresholding by optimizing a single decay time (Td) instead of multiple current thresholds. Using a PDVT-10 device, we demonstrate the first system that leverages the same PPC dynamics for both sensor-level preprocessing and physical reservoir computing. This integrated system achieved 96.54% accuracy on the Human Protein Atlas image recognition task, surpassing traditional hardware-based and software-based methods. This work redefines physical ‘defects’ as tunable computational resources, paving the way for developing minimalist and energy-efficient in-sensor computing systems.

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Article information

Article type
Paper
Submitted
16 Nov 2025
Accepted
20 Feb 2026
First published
21 Feb 2026

J. Mater. Chem. C, 2026, Accepted Manuscript

Persistent Photoconductivity Enables In-Sensor Binarization and Reservoir Computing in a Single Organic Phototransistor

H. Wang, H. Fan, W. Chen, W. Su, S. Weng, Z. Zou, X. Zhou, C. Wu, T. Guo and Y. Zhang, J. Mater. Chem. C, 2026, Accepted Manuscript , DOI: 10.1039/D5TC04070A

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