Thermal Dehydration of Swollen Heterogeneous Soft Materials

Abstract

The dehydration of bi-layer soft materials under temperature variations is a key process in applications such as biomedical devices and responsive hydrogels. This study develops a multiphysics model to investigate the coupled thermo-hydro-mechanical behavior of bi-domain materials. We present the governing equations capturing heat transfer, moisture diffusion, and mechanical deformation across two distinct material domains. Numerical simulations reveal that temperature gradients induce differential dehydration rates, leading to localized stresses and domain-specific shrinkage. Key findings include critical temperature thresholds, wet-bulb effect and the role of domain interface properties in material stability. These results provide insights into controlling the shape morphing of thermally responsive soft materials via tailored dehydration conditions.

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Article information

Article type
Paper
Submitted
22 Dec 2025
Accepted
02 Apr 2026
First published
02 Apr 2026

Soft Matter, 2026, Accepted Manuscript

Thermal Dehydration of Swollen Heterogeneous Soft Materials

M. Curatolo, G. Tomassetti, R. van der Sman and L. Teresi, Soft Matter, 2026, Accepted Manuscript , DOI: 10.1039/D5SM01263E

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