We report a catalyst-free, one-step strategy utilizing double dielectric barrier discharge to convert CH4 and H2O into light alcohols under ambient conditions, achieving 8 % methane conversion and 70 % light alcohol selectivity. Mechanistic analysis verifies that the dominant pathway for alcohol formation is the direct coupling of alkyl and hydroxyl radicals.
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Z. Gao, D. Li, Y. Yang, C. Wu, L. Wang, Z. Cui, L. Hua, H. Li, C. Peng, D. Deng and Y. Yi, Green Chem., 2026, Accepted Manuscript , DOI: 10.1039/D6GC01413E
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