Herein, a comparative investigation into the π-extension effect on a MR framework was conducted via heteroatom doping engineering. The as-synthesized emitters CzBNNO and CzBNBO both exhibited EQEs > 30%. However, they differ significantly in SRCT/LRCT dominance, which causes distinct discrepancies in spectral broadening and emission peak positions.
J. Li, Z. Cheng, S. Zhang, Y. Wang, H. Wang, J. Zhou, W. Gao, L. Qu, Z. Zhu, J. Yu, J. Ye and K. Wang, Phys. Chem. Chem. Phys., 2026, Accepted Manuscript , DOI: 10.1039/D5CP04299B
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