Modulation of spatial Raman gain induced by Laguerre–Gaussian vortex beams

Abstract

Electromagnetically induced transparency (EIT) provides a powerful platform for coherent control of optical properties in atomic media. Building upon this framework, we investigate a microwave-assisted closed-loop three-level atomic system driven by a Laguerre–Gaussian (LG) control beam and a Gaussian probe field. The present work emphasizes the spatial modulation mechanisms of Raman gain. Using the density matrix formalism, we numerically solve the steady-state equations to obtain two-dimensional maps and cross-sectional profiles of Raman gain.The results reveal that three key parameters—the orbital angular momentum (OAM) of the LG beam, the single-photon detuning, and the relative phase of the control fields—jointly determine the spatial morphology of the gain. Specifically, variations in OAM induce transitions from asymmetric single-lobe to symmetric multi-lobed gain structures; detuning modifies the gain intensity and spatial complexity; and relative phase produces rotational and mirror-symmetric transformations in the distribution.This study represents the first systematic analysis of spatial Raman gain modulation in a closed-loop three-level system, highlighting the strong capability of structured light to precisely tailor nonlinear gain processes. The results not only extend the theoretical framework of previous studies, but also provide a new theoretical basis for the design of spatial selective optical amplification, structured light field engineering and advanced nonlinear optical devices.

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Article information

Article type
Paper
Submitted
18 Sep 2025
Accepted
05 Jan 2026
First published
06 Jan 2026

Phys. Chem. Chem. Phys., 2026, Accepted Manuscript

Modulation of spatial Raman gain induced by Laguerre–Gaussian vortex beams

Q. MING and Z. Fu, Phys. Chem. Chem. Phys., 2026, Accepted Manuscript , DOI: 10.1039/D5CP03598H

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