A one-dimensional (1D) coordination tape with a ladder topology featuring pentagonal bipyramidal cobalt(II) centers was synthesized and magnetically characterized. Magnetic studies combined with ab initio calculations reveal the large easy-plane magnetic anisotropy of the tape with field-induced single-ion magnet (SIM) property, which renders this coordination tape the first seven-coordinate SIM tape.
M. Cai, A. P. singh, Z. Xu, D. Shao, S. Zhang, J. Yang, B. Zhao and S. K. Singh, CrystEngComm, 2026, Accepted Manuscript , DOI: 10.1039/D6CE00257A
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