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Constructing efficient electron transport channels in metal-organic frameworks (MOFs) is critical for boosting peroxymonosulfate (PMS) activation. We fabricated Co-doped MIL-101(Fe)-NH₂ catalyst, where Fe-Co orbital coupling constructs an electron pump for directional electron transfer to boost PMS activation and 1 O2mediated antibiotic degradation.
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Z. Chen, Y. Cui, L. Yang, R. Wang, X. Pan and F. Jiang, Chem. Commun., 2026, Accepted Manuscript , DOI: 10.1039/D6CC02401G
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