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A π-extended nonbenzenoid perylene (Pery-56) was constructed via ring-fusion strategy at both its bay and peri positions. As a result, it features a moderately lower bandgap, broad visible-NIR absorption (525-950 nm) with λmax around 700 nm and reversible redox behavior, with the cationic radical and anionic radical being thoroughly studied.
L. Zhou, Y. Bai, Y. Zhao, G. Liu, B. Rao, Z. Zhang and Q. Wang, Chem. Commun., 2026, Accepted Manuscript , DOI: 10.1039/D6CC02382G
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