Single-atom Pd anchored on In-MIL-68-bpy enables selective Photothermal catalysis oxidation of CH4 to HCHO in water. The Pd-N site promotes O2 activation and regulates reactive oxygen species generation, affording an HCHO formation rate of 1.9 mmol gcat-1 h-1 at 120 °C while suppressing deep oxidation to CO2.
S. Zhou, Z. Bao, S. Chen, X. Tian, H. Song, G. Li and H. Zhang, Chem. Commun., 2026, Accepted Manuscript , DOI: 10.1039/D6CC01599A
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