A molecular-to-atomic transformation of Co(PPh₃)₂Cl₂ on a covalent triazine polymer through carbonization yields Co-N₂P₂ single-atom sites on carbon matrix. The synergistic P/N coordination fine-tunes the Co electronic structure, enabling highly efficient α-alkylation of aromatic ketones.
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N. Anbuselvan, S. Sivaprakash, D. Sneha, B. Ghosh, D. Suresh and A. J. Amali, Chem. Commun., 2026, Accepted Manuscript , DOI: 10.1039/D6CC00398B
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