The coupling between the spin state and the complex motion of the individual alkyl chains results in a unique thermal hysteresis exhibiting an "inverted” loop. Specifically, the high-spin (HS) ￫ low-spin (LS) transition upon cooling to occur at a higher temperature than the LS ￫ HS transition upon heating.
A. Tołoczko, M. Kaźmierczak, V. Maliuzhenko, M. Siczek, M. Weselski and R. Bronisz, Chem. Commun., 2026, Accepted Manuscript , DOI: 10.1039/D6CC00357E
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