Amino-Bridged Quantum Dots/Covalent Organic Frameworks S-Scheme Heterojunction for Photocatalytic Overall Water Splitting
Abstract
An amino-bridged CdS/COF S-scheme heterojunction is constructed via molecular interfacial engineering. This design enhances charge separation while preserving strong redox capabilities. It prolongs carrier lifetime by 3.4-fold and boosts overall water splitting performance over 10-fold without sacrificial agents, highlighting the pivotal role of precise interface engineering.
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