Herein, we report a Lewis acid switching strategy that enables programmable selectivity between kinetically controlled N1 alkylation and thermodynamically favored N2 alkylation using α-hydroxyl diazo compounds as versatile electrophiles.
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J. Jiang, J. Zhang, N. Huang, H. Xu, X. Liu, J. Li, X. Zhou, J. Zhao and P. Li, Chem. Commun., 2026, Accepted Manuscript , DOI: 10.1039/D5CC07167D
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