Issue 6, 2025

Shear thickening inside elastic open-cell foams under dynamic compression

Abstract

We measure the response of open-cell polyurethane foams filled with a dense suspension of fumed silica particles in polyethylene glycol at compression speeds spanning several orders of magnitude. The gradual compressive stress increase of the composite material indicates the existence of shear rate gradients in the interstitial suspension caused by wide distributions in pore sizes in the disordered foam network. The energy dissipated during compression scales with an effective internal shear rate, allowing for the collapse of three data sets for different pore-size foams. When scaled by this effective shear rate, the most pronounced energy increase coincides with the effective shear rate corresponding to the onset of shear thickening in our bulk suspension. Optical measurements of the radial deformation of the foam network and of the suspension flow under compression provide additional insight into the interaction between shear thickening fluid and foam. This optical data, combined with a simple model of a spring submerged in viscous flow, illustrates the dynamic interaction of viscous drag with foam elasticity as a function of compression rate, and identifies the foam pore size distribution as a critically important model parameter. Taken together, the stress measurements, dissipated energy, and relative motion of the fluid and the foam can be rationalized by knowing the pore size distribution and the average pore size of the foam.

Graphical abstract: Shear thickening inside elastic open-cell foams under dynamic compression

Supplementary files

Article information

Article type
Paper
Submitted
30 Sep 2024
Accepted
08 Jan 2025
First published
14 Jan 2025
This article is Open Access
Creative Commons BY license

Soft Matter, 2025,21, 1192-1202

Shear thickening inside elastic open-cell foams under dynamic compression

S. M. Livermore, A. Pelosse, M. van der Naald, H. Kim, S. Atis and H. M. Jaeger, Soft Matter, 2025, 21, 1192 DOI: 10.1039/D4SM01144A

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