e-Methanation with a spiral catalyst: optimized thermal management and long-term stability

Abstract

This study explores the development of a Joule-heated reaction field utilizing an electrically driven spiral-shaped catalyst for efficient CO₂ methanation. Infrared thermal imaging in an uninsulated reactor reveals a rapid and uniform temperature rise along the spiral structure. With a 10 W input, CO₂ conversion reached 80%, while 75% conversion was maintained even at 5 W. The catalyst's twist angle played a crucial role in optimizing heat transfer and CO₂ conversion by enhancing swirl flow. Long-term stability tests at 5 W demonstrated sustained methane production over 50 hours at 350 °C, highlighting the catalyst's durability and energy efficiency.