Here, acceptorless dehydrogenative aromatization of cyclohexyl rings via benzylic C–H bond activation has been achieved using a supported Pd nanoparticle catalyst. Especially, in-situ formed Pd(0) nanoparticles from Pd hydroxide species during the dehydrogenation reactions showed high catalytic performance and a wide substrate scope.
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Q. Yu, T. Yatabe, M. Takehiro and K. Yamaguchi, Chem. Commun., 2025, Accepted Manuscript , DOI: 10.1039/D5CC05200A
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