High throughput screening of high entropy spinel electrolytes for multivalent batteries

Mahesh J. Dheerasinghe; Yi Gan; Lin Wang; Yufang He; Zhengda He; Gui-Liang Xu; Yang Zhao; Bin Ouyang

doi:10.1039/D5CC02095F

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High throughput screening of high entropy spinel electrolytes for multivalent batteries†

Mahesh J. Dheerasinghe,‡^a Yi Gan,‡^b Lin Wang,^a Yufang He,

^a Zhengda He,^a Gui-Liang Xu,

^c Yang Zhao

*^b and Bin Ouyang

*^a

Author affiliations

* Corresponding authors

^a Department of Chemistry and Biochemistry, Florida State University, Tallahassee, FL, USA
E-mail: bouyang@fsu.edu

^b Department of Mechanical and Materials Engineering, The University of Western Ontario, Canada

^c Chemical Sciences and Engineering Division, Argonne National Laboratory, Lemont, IL, USA

Abstract

High-entropy (HE) design emerged as a promising path for discovering multivalent superionic conductors. This work provides a computational exploration of the synthesizability of HE spinel-based electrolytes among the typical chemical space. Design principles have been established, while experimental synthesis has supported the stability rules predicted by computational data.

This article is part of the themed collection: Chemistry at the Forefront of the Sustainable Energy Transition

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DOI: https://doi.org/10.1039/D5CC02095F
Article type: Communication
Submitted: 14 Apr 2025
Accepted: 16 Jun 2025
First published: 19 Jun 2025
This article is Open Access

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Chem. Commun., 2025, Advance Article

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High throughput screening of high entropy spinel electrolytes for multivalent batteries

M. J. Dheerasinghe, Y. Gan, L. Wang, Y. He, Z. He, G. Xu, Y. Zhao and B. Ouyang, Chem. Commun., 2025, Advance Article , DOI: 10.1039/D5CC02095F

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Chemical Communications

High throughput screening of high entropy spinel electrolytes for multivalent batteries†

Abstract

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High throughput screening of high entropy spinel electrolytes for multivalent batteries

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