Issue 60, 2025

Dual-component modulation strategy for enhancing interfacial compatibility in 4.6 V LRMO-based solid-state lithium metal batteries

Abstract

Solid-state lithium metal batteries with a Li-rich manganese oxide (LRMO) cathode suffer from challenges in interfacial compatibility. This study improves the interface between a PVC-based gel electrolyte and electrodes via dual-component modulation. The optimized electrolyte exhibits high oxidation stability and facilitates the formation of inorganic-rich interphases, contributing to the long-term stability of the interface. Therefore, the 4.6 V Li|LRMO cells operate stably for 100 cycles at 0.2C, delivering an initial capacity of 215.2 mA h gāˆ’1 and average coulombic efficiency of 99.55%.

Graphical abstract: Dual-component modulation strategy for enhancing interfacial compatibility in 4.6 V LRMO-based solid-state lithium metal batteries

Supplementary files

Article information

Article type
Communication
Submitted
31 Mar 2025
Accepted
14 Jun 2025
First published
23 Jun 2025

Chem. Commun., 2025,61, 11239-11242

Dual-component modulation strategy for enhancing interfacial compatibility in 4.6 V LRMO-based solid-state lithium metal batteries

M. Wang, L. Xu, J. Tang, H. Ying, G. Han and Y. Shi, Chem. Commun., 2025, 61, 11239 DOI: 10.1039/D5CC01807B

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