Issue 31, 2025
From the journal:

Chemical Communications

One-pot synthesis of a highly active single-atom Pd catalyst for the Heck reaction†

Hui Teng,a   Qingyun Zhi,a   Yiming Zhang,a   Chengyou Zheng,a   Jie Chen,a   Zhenjiang Liang,a   Xinghua Yu, ORCID logo b   Yujun Zhang*ab  and  Junmin Zhang ORCID logo *a  

* Corresponding authors

a International Joint Research Center for Molecular Science, College of Chemistry and Environmental Engineering, Shenzhen Children's Hospital, Clinical Medical College of Shenzhen University, Shenzhen University, Shenzhen, P. R. China
E-mail: zhangjm@szu.edu.cn

b Department of Urology & Andrology, Sir Run Run Shaw Hospital, Zhejiang University School of Medicine, Hangzhou, Zhejiang, P. R. China
E-mail: zhangyujun@zju.edu.cn

Abstract

A two-dimensional nitrogen-doped graphene-supported palladium single-atom catalyst (Pd SACs/NG) was successfully, precisely and concisely synthesized by a one-pot method. We report for the first time that 2D Pd SACs/NG oriented towards the Heck reaction achieved catalytic efficiency with a TON up to 133 256, significantly outperforming the commercial Pd(CH3COO)2 and Pd/C catalysts, surpassing previous reports.

Graphical abstract: One-pot synthesis of a highly active single-atom Pd catalyst for the Heck reaction

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Article information

DOI
https://doi.org/10.1039/D5CC00796H
Article type
Communication
Submitted
13 Feb 2025
Accepted
14 Mar 2025
First published
14 Mar 2025

Chem. Commun., 2025,61, 5770-5773

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One-pot synthesis of a highly active single-atom Pd catalyst for the Heck reaction

H. Teng, Q. Zhi, Y. Zhang, C. Zheng, J. Chen, Z. Liang, X. Yu, Y. Zhang and J. Zhang, Chem. Commun., 2025, 61, 5770 DOI: 10.1039/D5CC00796H

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