Issue 32, 2025

Promoted exciton transport in organic semiconductors by triplet-state manipulation

Abstract

Efficient excited-state transport is essential for the optimal performance of photoelectronic devices, which, however, is very limited in organic semiconductors (OSCs) due to the presence of poorly diffusive triplet-states. Herein, we report a bridging group enabled triplet-state manipulation strategy for suppressing the intersystem crossing (ISC) and thereby realizing a promoted and directional singlet-state exciton transport in anthracene derivative-based OSCs. Furthermore, this approach is demonstrated to be applicable to various anthracene derivatives, such as bridged anthracene–benzothiophene and anthracene–benzene systems, suggesting its broad generalizability for optimizing the exciton/energy transport properties of OSCs.

Graphical abstract: Promoted exciton transport in organic semiconductors by triplet-state manipulation

Supplementary files

Article information

Article type
Communication
Submitted
22 Jan 2025
Accepted
13 Mar 2025
First published
19 Mar 2025

Chem. Commun., 2025,61, 6002-6005

Promoted exciton transport in organic semiconductors by triplet-state manipulation

L. Meng, C. Zhao, F. Li, J. Liu, X. Yan, Y. Wei, T. Yang, X. Zhang, L. Jiang, Z. Lu, Q. Sun, W. Tian and S. Jin, Chem. Commun., 2025, 61, 6002 DOI: 10.1039/D5CC00416K

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