Emergent multi-field interaction in a magnetic quasi-two-dimensional WSe2/SrCoO2.5/2DEG heterojunction

Abstract

WSe2-based heterostructures are extensively enhanced by dielectric and interfacial engineering for high-performance photodetector. However, it is difficult to integrate the magnetic 3D thin film on the 2D Van der Waals heterostructure. In this study, a magnetic quasi-two-dimensional p-WSe2/n-2DEG heterostructures with a inserted expitial SrCoO2.5 thin film are fabricated, and the p-n heterojunction formed via Ar+-ion-bombardment process. The fabricated device with a typical long depletion region responds to a broad spectral range from 447-808 nm within the wide temperature range of 10-300 K. Under the dark and light illumination, the magneto-optical response can be realized due to the self-charging process in the device. Furthermore, the adjustable multistate can be expected under multi-field interaction on the heretojunction, which can be controlled by the control signal as the light ON/OFF switching, bias, and magnetic field. Based on the experimental results and process simulation, it is demonstrated that the heterojunction with an optimized magnetic SrCoO2.5 design holds promise as a multimode logic gate, which can be implemented with complementary 2D/3D semiconductor design and fabrication processes.

Supplementary files

Article information

Article type
Paper
Submitted
06 Jun 2024
Accepted
06 Jul 2024
First published
08 Jul 2024

J. Mater. Chem. C, 2024, Accepted Manuscript

Emergent multi-field interaction in a magnetic quasi-two-dimensional WSe2/SrCoO2.5/2DEG heterojunction

X. Zhang, C. Xu, G. Sun, K. Li, H. Yang, G. Liu, Y. Jiang, J. Gao, H. Lu, R. Zhao and W. Tian, J. Mater. Chem. C, 2024, Accepted Manuscript , DOI: 10.1039/D4TC02341B

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