Issue 25, 2024

Redox-neutral zinc-catalyzed cascade [1,4]-H shift/annulation of diaziridines with donor–acceptor aziridines

Abstract

The coupling of diaziridines with donor–acceptor aziridines (DAAs) has been achieved using Zn-catalysis to furnish imidazopyrazole-4,4-dicarboxylates via [1,4]-hydride shift. The use of Zn-catalysis, [1,4]-hydride shift, natural product modification and a late-stage molecular docking study are important practical features.

Graphical abstract: Redox-neutral zinc-catalyzed cascade [1,4]-H shift/annulation of diaziridines with donor–acceptor aziridines

Supplementary files

Article information

Article type
Communication
Submitted
16 Jan 2024
Accepted
23 Feb 2024
First published
23 Feb 2024

Chem. Commun., 2024,60, 3441-3444

Redox-neutral zinc-catalyzed cascade [1,4]-H shift/annulation of diaziridines with donor–acceptor aziridines

S. Samantaray, P. K. Maharana, S. Kar, S. Saha and T. Punniyamurthy, Chem. Commun., 2024, 60, 3441 DOI: 10.1039/D4CC00226A

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