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Abstract | Cited by

The frustrated Lewis pair (FLP) site of (Ce, Ce)-O on the CeO2(110) surface undergoes reconstruction to form (La, Ce)-O upon La-doping. The FLP site of (La, Ce)-O with the tailored local Lewis acid–base property and increased spatial distance between the Lewis acid and base facilitates the tandem transformation of styrene and CO2 through the weakened adsorption of CO2 while maintaining activation.

Graphical abstract: Regulation of frustrated Lewis pairs on CeO2 facilitates tandem transformation of styrene and CO2

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