Issue 11, 2022

Elliptic dichroism in strong-field ionization of atoms subjected to tailored laser fields

Abstract

The differential ionization rate for strong-field ionization by tailored laser fields of atomic systems averaged over the magnetic quantum number satisfies particular inversion and reflection symmetries. The symmetries of the elliptic-dichroism parameter, which is related to the change of sign of the ellipticity of the laser field, are considered in detail, with particular emphasis on high-order above-threshold ionization. The general results are illustrated by the examples of an elliptically polarized laser field and a bi-elliptical orthogonally polarized two-color (BEOTC) field. For the BEOTC field the differential ionization rate and the elliptic-dichroism parameter are investigated for the ω–2ω and ω–3ω field combinations and for various relative phases between the laser-field components. The inversion and reflection symmetries of the photoelectron momentum distribution in the polarization plane of the field depend on the parities of r and s in the -- BEOTC field combination and on the relative phase between the field components. We suggest that, by analyzing the symmetry properties of the measured momentum distribution of the elliptic-dichroism parameter, one can identify the mechanism of strong-field ionization. If the rescattering mechanism is dominant one can use these distributions to obtain information about the atomic and molecular structure and dynamics.

Graphical abstract: Elliptic dichroism in strong-field ionization of atoms subjected to tailored laser fields

Article information

Article type
Paper
Submitted
13 Nov 2021
Accepted
23 Feb 2022
First published
25 Feb 2022

Phys. Chem. Chem. Phys., 2022,24, 7014-7027

Elliptic dichroism in strong-field ionization of atoms subjected to tailored laser fields

W. Becker and D. B. Milošević, Phys. Chem. Chem. Phys., 2022, 24, 7014 DOI: 10.1039/D1CP05209H

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