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Issue 3, 2021
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Increased residual lithium compounds guided design for green recycling of spent lithium-ion cathodes

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Abstract

Recycling of spent lithium-ion batteries has recently become a critical issue based on environmental concerns and a desire to reutilize resources. Among the existing recycling strategies, direct regeneration is largely encouraged from an economic and environmental perspective. However, current procedures used to separate the active cathode materials from the aluminum foil have some limitations for direct regeneration because they either destroy the structure of the cathode or use too many toxic and expensive reagents. Hence, we conducted comprehensive research on the microstructural evolution of the LiNi1−xyCoxMnyO2 degraded electrode and then proposed a targeted method to recycle the spent cathode materials based on the increased residual lithium compounds. This separation process involves no other reagents but water, and toxic organic solvents, complicated processes, and waste treatments are unnecessary compared with the existing pretreatment strategies. Moreover, the separated cathodes are suitable for direct regeneration. Satisfactory capacity recovery of the cathode was achieved via simple sintering. Such a recycling process enables a sustainable closed-loop for the spent cathodes and provides new inspiration for the design of LIB recycling.

Graphical abstract: Increased residual lithium compounds guided design for green recycling of spent lithium-ion cathodes

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Supplementary files

Article information


Submitted
15 Dec 2020
Accepted
01 Feb 2021
First published
02 Feb 2021

Energy Environ. Sci., 2021,14, 1461-1468
Article type
Paper

Increased residual lithium compounds guided design for green recycling of spent lithium-ion cathodes

M. Fan, X. Chang, Y. Guo, W. Chen, Y. Yin, X. Yang, Q. Meng, L. Wan and Y. Guo, Energy Environ. Sci., 2021, 14, 1461
DOI: 10.1039/D0EE03914D

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