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Synergistic performance of a sub-nanoscopic cobalt and imidazole grafted porous organic polymer for CO2 fixation to cyclic carbonates under ambient pressure without a co-catalyst

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Abstract

A facile, single-step development strategy of a sub-nanoscopic Lewis acidic Co and basic imidazole grafted porous organic polymer is reported. The synergistic activation of an epoxide and CO2 by the Lewis pairs present in the material manifested their rapid conversion to cyclic carbonates under ambient pressure with high yield, selectivity, and TOF.

Graphical abstract: Synergistic performance of a sub-nanoscopic cobalt and imidazole grafted porous organic polymer for CO2 fixation to cyclic carbonates under ambient pressure without a co-catalyst

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Article information


Submitted
11 Mar 2020
Accepted
30 Apr 2020
First published
30 Apr 2020

J. Mater. Chem. A, 2020, Advance Article
Article type
Communication

Synergistic performance of a sub-nanoscopic cobalt and imidazole grafted porous organic polymer for CO2 fixation to cyclic carbonates under ambient pressure without a co-catalyst

J. Chakraborty, I. Nath, S. Song, C. Kao and F. Verpoort, J. Mater. Chem. A, 2020, Advance Article , DOI: 10.1039/D0TA02821E

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