Self similarity of liquid droplet coalescence in a quasi-2D free-standing liquid-crystal film

Abstract

Coalescence of droplets is an ubiquitous phenomenon in chemical, physical and biological systems. The process of merging of liquid objects has been studied during the past years experimentally and theoretically in different geometries. We introduce a unique system that allows a quasi two-dimensional description of the coalescence process: Micrometer-sized flat droplets in freely suspended smectic liquid-crystal films. We find that the bridge connecting the droplets grows linearly in time during the initial stage of coalescence, both with respect to its height and lateral width. We also verify self-similar dynamics of the bridge during the first stage of coalescence. We compare our results with a model based on the thin sheet equations. Our experiments confirm that the most important geometrical parameter influencing the coalescence rate is the contact angle of the droplets.