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Immobilized BiCl3@Bi@g-C3N4 on one-dimensional multi-channel carbon fibers as heterogeneous catalyst for efficient CO2 cycloaddition reaction

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Abstract

A novel heterogeneous catalyst (BBCNC), where the Bi, BiCl3 and g-C3N4 were deposited on one-dimensional multi-channel carbon fibers (CNFs), was developed and characterized. And it was found that Bi3+ could be reduced to Bi by the substance from the thermal polycondensation of melamine and the carrier CNFs. The Lewis acid and base sites enabled a synergistically catalytic cycloaddition reaction of CO2 with high catalytic conversion and selectivity.

Graphical abstract: Immobilized BiCl3@Bi@g-C3N4 on one-dimensional multi-channel carbon fibers as heterogeneous catalyst for efficient CO2 cycloaddition reaction

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Article information


Submitted
17 Feb 2020
Accepted
11 Jun 2020
First published
11 Jun 2020

Inorg. Chem. Front., 2020, Advance Article
Article type
Research Article

Immobilized BiCl3@Bi@g-C3N4 on one-dimensional multi-channel carbon fibers as heterogeneous catalyst for efficient CO2 cycloaddition reaction

R. He, D. Zhang, G. Xu, C. Li and J. Bai, Inorg. Chem. Front., 2020, Advance Article , DOI: 10.1039/D0QI00207K

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