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Sesquiterpene synthases for bungoene, pentalenene and epi-isozizaene from Streptomyces bungoensis

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Abstract

A sesquiterpene synthase from Streptomyces bungoensis was characterised and produces the new compound bungoene. The enzyme mechanism was deeply investigated using isotopically labelled substrates. Two other enzymes from S. bungoensis made epi-isozizaene and pentalenene. Synthetic oxidative chemistry towards structurally related fusagramineol and pentalenal was explored.

Graphical abstract: Sesquiterpene synthases for bungoene, pentalenene and epi-isozizaene from Streptomyces bungoensis

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Submitted
23 Mar 2020
Accepted
01 Apr 2020
First published
02 Apr 2020

Org. Biomol. Chem., 2020, Advance Article
Article type
Communication

Sesquiterpene synthases for bungoene, pentalenene and epi-isozizaene from Streptomyces bungoensis

L. Lauterbach and J. S. Dickschat, Org. Biomol. Chem., 2020, Advance Article , DOI: 10.1039/D0OB00606H

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