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Synthesis of α-enaminones from cyclic ketones and anilines using oxoammonium salt as an oxygen transfer reagent

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Abstract

A convenient and straightforward transformation of cyclic ketones with anilines at room temperature has been developed using oxoammonium salt TEMPO+PF6 as an oxidant. This method enabled the synthesis of a broad range of α-enaminones. The 18O-labeling experiment demonstrated that oxoammonium salt served as the oxygen transfer reagent.

Graphical abstract: Synthesis of α-enaminones from cyclic ketones and anilines using oxoammonium salt as an oxygen transfer reagent

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Article information


Submitted
08 Nov 2019
Accepted
02 Jan 2020
First published
07 Jan 2020

Green Chem., 2020, Advance Article
Article type
Communication

Synthesis of α-enaminones from cyclic ketones and anilines using oxoammonium salt as an oxygen transfer reagent

B. Xu, Y. Shang, X. Jie, X. Zhang, J. Kan, S. L. Yedage and W. Su, Green Chem., 2020, Advance Article , DOI: 10.1039/C9GC03845K

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