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A new cobalt metal–organic framework as a substrate for Pd nanoparticles applied in high-efficiency nitro phenol degradation and cinnamaldehyde hydrogenation

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Abstract

In recent years, attributed to the excellent catalytic performance of precious metal materials, metal nanoparticles@MOF catalyst has been a popular research direction. Herein, we have synthesized a new 3D cobalt metal–organic framework [Co(TATAB)(344-pytpy)·DMF]n(H3TATAB = 4,4′,4″-s-triazine-1,3,5-triyltri-p-aminobenzoic acid; 344-pytpy = 4′-(3-pyridyl)-4,2′:6′,4″-terpyridine)(1)(P1) by solvothermal method. Its crystal structure was determined with single-crystal X-ray diffraction (SC-XRD) techniques. The final composite Pd-NPs@1 catalyst was synthesized by a reduction method. The catalyst showed high catalytic performance and high recycling stability for nitrophenol degradation and cinnamaldehyde hydrogenation reaction.

Graphical abstract: A new cobalt metal–organic framework as a substrate for Pd nanoparticles applied in high-efficiency nitro phenol degradation and cinnamaldehyde hydrogenation

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Article information


Submitted
16 Oct 2019
Accepted
10 Dec 2019
First published
11 Dec 2019

Dalton Trans., 2020, Advance Article
Article type
Paper

A new cobalt metal–organic framework as a substrate for Pd nanoparticles applied in high-efficiency nitro phenol degradation and cinnamaldehyde hydrogenation

Z. Liu, L. Ning, K. Wang, L. Feng, W. Gu and X. Liu, Dalton Trans., 2020, Advance Article , DOI: 10.1039/C9DT04051J

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