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Selective formic acid dehydrogenation at low temperature over a RuO2/COF pre-catalyst synthesized on the gram scale

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Abstract

A pre-catalyst, consisting of RuO2 nanoparticles and clusters anchored on TpBD-Me2 COF, was synthesized. During catalytic formic acid dehydrogenation, RuO2 undergoes in situ reduction to metallic Ru, forming an active and selective catalyst, which outperforms the commercial Ru–C catalyst. The chemical structure of the COF supporting material is maintained during stability testing.

Graphical abstract: Selective formic acid dehydrogenation at low temperature over a RuO2/COF pre-catalyst synthesized on the gram scale

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Article information


Submitted
24 Jan 2020
Accepted
25 Feb 2020
First published
25 Feb 2020

Catal. Sci. Technol., 2020, Advance Article
Article type
Communication

Selective formic acid dehydrogenation at low temperature over a RuO2/COF pre-catalyst synthesized on the gram scale

L. P. L. Gonçalves, D. B. Christensen, M. Meledina, L. M. Salonen, D. Y. Petrovykh, E. Carbó-Argibay, J. P. S. Sousa, O. S. G. P. Soares, M. F. R. Pereira, S. Kegnæs and Y. V. Kolen'ko, Catal. Sci. Technol., 2020, Advance Article , DOI: 10.1039/D0CY00145G

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