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Real-time monitoring of surface acetone enolization and aldolization

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Abstract

We report the identification of acetone enolate and its subsequent aldolization. The real-time evolution of surface species monitored by in situ DRIFTS of surface acetone (-d6) reactions shows clear spectroscopic evidence of the formation of acetone enolate and its subsequent aldolization via a dominant Eley–Rideal type mechanism on Zn1Zr10Oz.

Graphical abstract: Real-time monitoring of surface acetone enolization and aldolization

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Article information


Submitted
18 Nov 2019
Accepted
03 Jan 2020
First published
06 Jan 2020

Catal. Sci. Technol., 2020, Advance Article
Article type
Communication

Real-time monitoring of surface acetone enolization and aldolization

H. Li, J. Sun, G. Li, D. Wu and Y. Wang, Catal. Sci. Technol., 2020, Advance Article , DOI: 10.1039/C9CY02339A

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