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Structural characterization of molybdenum–dinitrogen complex as key species toward ammonia formation by dispersive XAFS spectroscopy

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Abstract

The structural characterization of a hardly-isolatable molybdenum–dinitrogen complex bearing a PNP-type pincer ligand, which is assumed to be a key reactive complex in the stoichiometric transformation of a molybdenum triiodide complex [MoI3(PNP)] into the corresponding molybdenum nitride complex under an atmospheric pressure of dinitrogen, was carried out by using dispersive XAFS.

Graphical abstract: Structural characterization of molybdenum–dinitrogen complex as key species toward ammonia formation by dispersive XAFS spectroscopy

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Article information


Submitted
16 Dec 2019
Accepted
22 Apr 2020
First published
23 Apr 2020

Phys. Chem. Chem. Phys., 2020, Advance Article
Article type
Communication

Structural characterization of molybdenum–dinitrogen complex as key species toward ammonia formation by dispersive XAFS spectroscopy

A. Yamamoto, K. Arashiba, S. Naniwa, K. Kato, H. Tanaka, K. Yoshizawa, Y. Nishibayashi and H. Yoshida, Phys. Chem. Chem. Phys., 2020, Advance Article , DOI: 10.1039/C9CP06761B

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