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Pd/Xiang-Phos-catalyzed enantioselective intermolecular carboheterofunctionalization of norbornene and norbornadiene

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Abstract

A highly enantioselective Pd/Xiang-Phos-catalyzed carbohetero-functionalization of norbornene is described, giving a direct access to various chiral norbornane-fused dihydrofurans and dihydro-pyrroles. This synthetic methodology provides the first example of asymmetric carboetherification of norbornene, and also tolerates norbornadiene well.

Graphical abstract: Pd/Xiang-Phos-catalyzed enantioselective intermolecular carboheterofunctionalization of norbornene and norbornadiene

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Submitted
21 Jul 2020
Accepted
15 Sep 2020
First published
18 Sep 2020

Chem. Commun., 2020, Advance Article
Article type
Communication

Pd/Xiang-Phos-catalyzed enantioselective intermolecular carboheterofunctionalization of norbornene and norbornadiene

M. Tao, W. Li and J. Zhang, Chem. Commun., 2020, Advance Article , DOI: 10.1039/D0CC04996D

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