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Issue 90, 2020
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Unravelling a long-lived ligand-to-metal cluster charge transfer state in Ce–TCPP metal organic frameworks

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Abstract

Metal organic frameworks (MOFs) have emerged as promising photocatalytic materials for solar energy conversion. However, a fundamental understanding of light harvesting and charge separation (CS) dynamics in MOFs remains underexplored, yet they are key factors that determine the efficiency of photocatalysis. Herein, we report the design and CS dynamics of the Ce–TCPP MOF using ultrafast spectroscopic methods.

Graphical abstract: Unravelling a long-lived ligand-to-metal cluster charge transfer state in Ce–TCPP metal organic frameworks

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Article information


Submitted
12 Jun 2020
Accepted
13 Oct 2020
First published
13 Oct 2020

Chem. Commun., 2020,56, 13971-13974
Article type
Communication

Unravelling a long-lived ligand-to-metal cluster charge transfer state in Ce–TCPP metal organic frameworks

S. Yang, W. Hu, J. Nyakuchena, C. Fiankor, C. Liu, E. D. Kinigstein, J. Zhang, X. Zhang and J. Huang, Chem. Commun., 2020, 56, 13971
DOI: 10.1039/D0CC04116E

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