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Dopamine polymer derived isolated single-atom sites metals/N-doped porous carbon for benzene oxidation

Abstract

Isolated single atom sites metals/nitrogen-doped porous carbon (ISAS M/NPC, M = Fe, Co, Ni) catalyst are successfully prepared by a top-down polymerization-pyrolysis-etching-activation (PPEA) strategy, which use dopamine as precursors. Due to the isolated single atom Fe active sites and porous structure, the ISAS Fe/NPC displayed a high benzene conversion up to 42.6% and nearly 100 % phenol selectivity.

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Article information


Submitted
21 May 2020
Accepted
23 Jun 2020
First published
24 Jun 2020

Chem. Commun., 2020, Accepted Manuscript
Article type
Communication

Dopamine polymer derived isolated single-atom sites metals/N-doped porous carbon for benzene oxidation

K. Wu, F. Zhan, R. Tu, W. (. Cheong, Y. Cheng, L. Zheng, W. Yan, Q. Zhang, Z. Chen and C. Chen, Chem. Commun., 2020, Accepted Manuscript , DOI: 10.1039/D0CC03620J

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