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Issue 53, 2020
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Zinc(ii)-catalyzed intramolecular hydroarylation-redox cross-dehydrogenative coupling of N-propargylanilines with diverse carbon pronucleophiles: facile access to functionalized tetrahydroquinolines

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Abstract

Zinc(II)-catalyzed intramolecular hydroarylation-redox cross-dehydrogenative coupling of N-propargylanilines with two types of carbon pronucleophiles (nitromethane as a sp3 carbon pronucleophile and phenylacetylenes as sp carbon pronucleophiles) proceeded to give the 2-substituted tetrahydroquinolines in good yields with 100% atomic utilization without any additional external oxidants.

Graphical abstract: Zinc(ii)-catalyzed intramolecular hydroarylation-redox cross-dehydrogenative coupling of N-propargylanilines with diverse carbon pronucleophiles: facile access to functionalized tetrahydroquinolines

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Supplementary files

Article information


Submitted
22 Apr 2020
Accepted
26 May 2020
First published
27 May 2020

Chem. Commun., 2020,56, 7333-7336
Article type
Communication

Zinc(II)-catalyzed intramolecular hydroarylation-redox cross-dehydrogenative coupling of N-propargylanilines with diverse carbon pronucleophiles: facile access to functionalized tetrahydroquinolines

G. Li, C. Wang, Y. Li, K. Shao, G. Yu, S. Wang, X. Guo, W. Zhao and H. Nakamura, Chem. Commun., 2020, 56, 7333
DOI: 10.1039/D0CC02921A

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