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Tandem approach to NOBIN analogues from arylhydroxylamines and diaryliodonium salts via [3,3]-sigmatropic rearrangement

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Abstract

Herein, we present a transition-metal free direct O-arylation of arylhydroxylamines employing diaryliodonium salts as arylation reagents to form transient N,O-diarylhydroxylamines that could subsequently undergo [3,3]-sigmatropic rearrangement and re-aromatization to afford structurally diverse NOBIN analogs in good to excellent yields under mild conditions.

Graphical abstract: Tandem approach to NOBIN analogues from arylhydroxylamines and diaryliodonium salts via [3,3]-sigmatropic rearrangement

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Article information


Submitted
24 Apr 2020
Accepted
10 Jun 2020
First published
19 Jun 2020

Chem. Commun., 2020, Advance Article
Article type
Communication

Tandem approach to NOBIN analogues from arylhydroxylamines and diaryliodonium salts via [3,3]-sigmatropic rearrangement

H. Yuan, Y. Du, F. Liu, L. Guo, Q. Sun, L. Feng and H. Gao, Chem. Commun., 2020, Advance Article , DOI: 10.1039/D0CC02919J

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